Here is the best charisma outfit that also offers the best protection:

Sharp Heavy Synth Chest Piece: +1
Sharp Heavy Synth Left Leg: +1
Sharp Heavy Synth Left Arm: +1
Sharp Heavy Synth Right Leg: +1
Sharp Heavy Synth Right Arm: +1
Trilby or Newsboy Cap: +1 (Accepts Ballistic Weave)
Green Shirt & Combat Boots: +1 (Accepts Ballistic Weave. Also comes with +1 Endurance)
Black-rim or Fashionable Glasses: +1

This outfit, equipped with Mark V ballistic weave, gives your character the following total bonuses:

Charisma: +8
Endurance: +1
Intelligence: +5
Energy Resistance: 230
Ballistic Resistance: 217

Consumables brings your Charisma up even further:

Beer (any type): +1
Grape Mentats: +5
X-cell: +2

For a total possible bonus of +8. X-cell is extremely rare, so don;t work it into your charisma build. Instead, reply on beer and Grape Mentats. You can craft the later at any chemistry station.

If you want more ballistic resistance at the expense of energy resistance, go with heavy robot armor.

You can use Summer Shorts in place of Green Shirt & Combat Boots. This will give you one extra point of Charisma. However, you cannot wear a chest armor piece over it. This removes your charisma bonus from the Sharp Chest, which makes it equal (in terms of charisma) to using the Green Shirt & Combat Boots. However, Summer Shorts do not accept ballistic weave. That along with the +1 Endurance bonus from the Green Shirt & Combat Boots makes the later item "best in slot" for a high Charisma build that also offers high end-game defense stats.

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